hello thank you for reading this question, i have a iron cored dc-ac transformer (relies on interrupter to constantly break circuit to induce induction in secondary coil) a brief and crude diagram can be found
If I understand correctly, you want to turn an old transformer into an electromagnet, and you want to use both windings in order to get the strongest possible field. First of all, you are going to need to modify the core: It needs a gap. In a perfect transformer, the lines of magnetic force would be entirely confined to the core.